diff --git a/appstate/remote_binding.go b/appstate/remote_binding.go
index e315d51..f460c56 100644
--- a/appstate/remote_binding.go
+++ b/appstate/remote_binding.go
@@ -115,6 +115,22 @@ func ConfigureRemoteBinding(model *vault.Model, input RemoteBindingInput) (Remot
 	}, nil
 }
 
+func RemoveRemoteBinding(model *vault.Model, binding RemoteBinding) error {
+	if model == nil {
+		return fmt.Errorf("model is required")
+	}
+	if strings.TrimSpace(binding.RemoteProfileID) == "" {
+		return fmt.Errorf("remote profile id is required")
+	}
+	if strings.TrimSpace(binding.CredentialEntryID) == "" {
+		return fmt.Errorf("credential entry id is required")
+	}
+
+	model.RemoveRemoteProfileByID(binding.RemoteProfileID)
+	model.RemoveEntryByID(binding.CredentialEntryID)
+	return nil
+}
+
 func normalizeSyncMode(mode SyncMode) SyncMode {
 	switch mode {
 	case SyncModeAutomaticOnOpenSave:
diff --git a/appstate/remote_binding_test.go b/appstate/remote_binding_test.go
index de0e021..22b6ab9 100644
--- a/appstate/remote_binding_test.go
+++ b/appstate/remote_binding_test.go
@@ -212,3 +212,39 @@ func TestConfigureRemoteBindingRejectsIncompleteInput(t *testing.T) {
 		})
 	}
 }
+
+func TestRemoveRemoteBindingRemovesProfileAndCredentialsFromVault(t *testing.T) {
+	t.Parallel()
+
+	model := vault.Model{
+		Entries: []vault.Entry{{
+			ID:       "remote-creds-1",
+			Title:    "WebDAV Sign-In",
+			Username: "tjulian",
+			Password: "token-1",
+		}},
+		RemoteProfiles: []vault.RemoteProfile{{
+			ID:      "family-webdav",
+			Name:    "Family Vault",
+			Backend: vault.RemoteBackendWebDAV,
+			BaseURL: "https://dav.example.invalid/remote.php/dav",
+			Path:    "files/family/keepass.kdbx",
+		}},
+	}
+
+	err := RemoveRemoteBinding(&model, RemoteBinding{
+		LocalVaultPath:    "/tmp/family.kdbx",
+		RemoteProfileID:   "family-webdav",
+		CredentialEntryID: "remote-creds-1",
+	})
+	if err != nil {
+		t.Fatalf("RemoveRemoteBinding() error = %v", err)
+	}
+
+	if got := len(model.RemoteProfiles); got != 0 {
+		t.Fatalf("len(RemoteProfiles) = %d, want 0", got)
+	}
+	if _, err := model.EntryByID("remote-creds-1"); !errors.Is(err, vault.ErrEntryNotFound) {
+		t.Fatalf("EntryByID(remote-creds-1) error = %v, want ErrEntryNotFound", err)
+	}
+}
diff --git a/appstate/state.go b/appstate/state.go
index 6533172..7dfdc7f 100644
--- a/appstate/state.go
+++ b/appstate/state.go
@@ -920,6 +920,26 @@ func (s *State) ConfigureRemoteBinding(input RemoteBindingInput) (RemoteBinding,
 	return binding, nil
 }
 
+func (s *State) RemoveRemoteBinding(binding RemoteBinding) error {
+	session, ok := s.Session.(MutableSession)
+	if !ok {
+		return fmt.Errorf("session is not mutable")
+	}
+
+	model, err := session.Current()
+	if err != nil {
+		return err
+	}
+
+	if err := RemoveRemoteBinding(&model, binding); err != nil {
+		return err
+	}
+
+	session.Replace(model)
+	s.Dirty = true
+	return nil
+}
+
 func (s *State) CreateGroup(name string) error {
 	session, ok := s.Session.(MutableSession)
 	if !ok {
diff --git a/appstate/state_test.go b/appstate/state_test.go
index 1da9d45..cab5a76 100644
--- a/appstate/state_test.go
+++ b/appstate/state_test.go
@@ -1168,6 +1168,46 @@ func TestConfigureRemoteBindingRequiresMutableSession(t *testing.T) {
 	}
 }
 
+func TestRemoveRemoteBindingRemovesVaultDataAndMarksDirty(t *testing.T) {
+	t.Parallel()
+
+	sess := &mutableStubSession{model: vault.Model{
+		Entries: []vault.Entry{{
+			ID:       "remote-creds-1",
+			Title:    "WebDAV Sign-In",
+			Username: "tjulian",
+			Password: "token-1",
+		}},
+		RemoteProfiles: []vault.RemoteProfile{{
+			ID:      "family-webdav",
+			Name:    "Family Vault",
+			Backend: vault.RemoteBackendWebDAV,
+			BaseURL: "https://dav.example.invalid/remote.php/dav",
+			Path:    "files/family/keepass.kdbx",
+		}},
+	}}
+	state := State{Session: sess}
+
+	err := state.RemoveRemoteBinding(RemoteBinding{
+		LocalVaultPath:    "/tmp/family.kdbx",
+		RemoteProfileID:   "family-webdav",
+		CredentialEntryID: "remote-creds-1",
+	})
+	if err != nil {
+		t.Fatalf("RemoveRemoteBinding() error = %v", err)
+	}
+
+	if !state.Dirty {
+		t.Fatal("Dirty = false, want true after RemoveRemoteBinding")
+	}
+	if got := len(sess.model.RemoteProfiles); got != 0 {
+		t.Fatalf("len(RemoteProfiles) = %d, want 0", got)
+	}
+	if _, err := sess.model.EntryByID("remote-creds-1"); !errors.Is(err, vault.ErrEntryNotFound) {
+		t.Fatalf("EntryByID(remote-creds-1) error = %v, want ErrEntryNotFound", err)
+	}
+}
+
 func TestLockClearsSelectionAndMakesVaultUnavailable(t *testing.T) {
 	t.Parallel()
 
diff --git a/main.go b/main.go
index c634376..ef447a6 100644
--- a/main.go
+++ b/main.go
@@ -296,6 +296,7 @@ type ui struct {
 	useSavedAdvancedSyncRemote           widget.Clickable
 	openSelectedVaultRemote              widget.Clickable
 	saveCurrentRemoteBinding             widget.Clickable
+	removeSelectedRemoteBinding          widget.Clickable
 	openSecuritySettings                 widget.Clickable
 	openRemotePrefsHelp                  widget.Clickable
 	closeAdvancedSync                    widget.Clickable
@@ -2646,6 +2647,14 @@ func (u *ui) remoteSyncSettingsShortcutLabel() string {
 	return "Remote Sync Settings"
 }
 
+func (u *ui) shouldShowRemoveRemoteSyncShortcut() bool {
+	return u.shouldShowRemoteSyncSettingsShortcut()
+}
+
+func (u *ui) removeRemoteSyncShortcutLabel() string {
+	return "Stop Using Remote Sync"
+}
+
 func (u *ui) shouldShowRemoteSyncSetupShortcut() bool {
 	if !u.hasOpenVault() || u.isVaultLocked() || u.state.Section != appstate.SectionEntries {
 		return false
@@ -2719,6 +2728,49 @@ func (u *ui) saveCurrentRemoteBindingAction() error {
 	return nil
 }
 
+func (u *ui) stripRecentRemoteBinding(binding appstate.RemoteBinding) {
+	localPath := strings.TrimSpace(binding.LocalVaultPath)
+	profileID := strings.TrimSpace(binding.RemoteProfileID)
+	credentialID := strings.TrimSpace(binding.CredentialEntryID)
+	for i := range u.recentRemotes {
+		record := &u.recentRemotes[i]
+		if strings.TrimSpace(record.LocalVaultPath) != localPath {
+			continue
+		}
+		if strings.TrimSpace(record.RemoteProfileID) != profileID {
+			continue
+		}
+		if strings.TrimSpace(record.CredentialEntryID) != credentialID {
+			continue
+		}
+		record.LocalVaultPath = ""
+		record.RemoteProfileID = ""
+		record.CredentialEntryID = ""
+		record.SyncMode = ""
+	}
+}
+
+func (u *ui) removeSelectedRemoteBindingAction() error {
+	binding, ok := u.selectedVaultRemoteBinding()
+	if !ok {
+		return fmt.Errorf("no saved remote sync target is selected")
+	}
+	if err := u.state.RemoveRemoteBinding(binding); err != nil {
+		return err
+	}
+	if err := u.state.Save(); err != nil {
+		return err
+	}
+	u.stripRecentRemoteBinding(binding)
+	u.selectedVaultRemoteProfileID = ""
+	u.selectedVaultRemoteCredentialEntryID = ""
+	u.selectedVaultRemoteSyncMode = appstate.SyncModeManual
+	u.remoteUsername.SetText("")
+	u.remotePassword.SetText("")
+	u.showStatusMessage("Remote sync is no longer set up for this vault.")
+	return nil
+}
+
 func (u *ui) saveCurrentRemoteBindingHeading() string {
 	return "Bind this local vault to the current remote target"
 }
@@ -4291,6 +4343,9 @@ func (u *ui) layout(gtx layout.Context) layout.Dimensions {
 	for u.saveCurrentRemoteBinding.Clicked(gtx) {
 		u.runAction("save remote binding", u.saveCurrentRemoteBindingAction)
 	}
+	for u.removeSelectedRemoteBinding.Clicked(gtx) {
+		u.runAction("remove remote sync binding", u.removeSelectedRemoteBindingAction)
+	}
 	for u.shareCurrentVault.Clicked(gtx) {
 		u.runAction("share vault", u.shareCurrentVaultAction)
 	}
@@ -6857,7 +6912,7 @@ func (u *ui) pathBar(gtx layout.Context) layout.Dimensions {
 			return children
 		}()...)
 	}
-	if !u.shouldShowDirectRemoteSyncShortcut() && !u.shouldShowRemoteSyncSetupShortcut() && !u.shouldShowRemoteSyncSettingsShortcut() {
+	if !u.shouldShowDirectRemoteSyncShortcut() && !u.shouldShowRemoteSyncSetupShortcut() && !u.shouldShowRemoteSyncSettingsShortcut() && !u.shouldShowRemoveRemoteSyncShortcut() {
 		return crumbBar(gtx)
 	}
 	children := []layout.FlexChild{
@@ -6885,6 +6940,14 @@ func (u *ui) pathBar(gtx layout.Context) layout.Dimensions {
 			return tonedButton(gtx, u.theme, &u.useSavedAdvancedSyncRemote, u.remoteSyncSettingsShortcutLabel())
 		}))
 	}
+	if u.shouldShowRemoveRemoteSyncShortcut() {
+		if u.shouldShowDirectRemoteSyncShortcut() || u.shouldShowRemoteSyncSetupShortcut() || u.shouldShowRemoteSyncSettingsShortcut() {
+			children = append(children, layout.Rigid(layout.Spacer{Height: unit.Dp(6)}.Layout))
+		}
+		children = append(children, layout.Rigid(func(gtx layout.Context) layout.Dimensions {
+			return tonedButton(gtx, u.theme, &u.removeSelectedRemoteBinding, u.removeRemoteSyncShortcutLabel())
+		}))
+	}
 	return layout.Flex{Axis: layout.Vertical}.Layout(gtx, children...)
 }
 
diff --git a/main_test.go b/main_test.go
index b95bbed..77a19ea 100644
--- a/main_test.go
+++ b/main_test.go
@@ -5904,6 +5904,41 @@ func TestUIRemoteSyncSettingsShortcutLabelUsesClearLanguage(t *testing.T) {
 	}
 }
 
+func TestUIShouldShowRemoveRemoteSyncShortcutForSavedBinding(t *testing.T) {
+	t.Parallel()
+
+	u := newUIWithModel("desktop", vault.Model{
+		Entries: []vault.Entry{{
+			ID:       "remote-creds-1",
+			Title:    "WebDAV Sign-In",
+			Username: "tjulian",
+			Path:     []string{"Crew", "Internet"},
+		}},
+		RemoteProfiles: []vault.RemoteProfile{{
+			ID:      "family-webdav",
+			Name:    "Family Vault",
+			Backend: vault.RemoteBackendWebDAV,
+			BaseURL: "https://dav.example.invalid/remote.php/dav",
+			Path:    "files/family/keepass.kdbx",
+		}},
+	})
+	u.state.Section = appstate.SectionEntries
+
+	if !u.shouldShowRemoveRemoteSyncShortcut() {
+		t.Fatal("shouldShowRemoveRemoteSyncShortcut() = false, want true when a saved binding exists")
+	}
+}
+
+func TestUIRemoveRemoteSyncShortcutLabelUsesClearLanguage(t *testing.T) {
+	t.Parallel()
+
+	u := newUIWithSession("desktop", &session.Manager{})
+
+	if got := u.removeRemoteSyncShortcutLabel(); got != "Stop Using Remote Sync" {
+		t.Fatalf("removeRemoteSyncShortcutLabel() = %q, want Stop Using Remote Sync", got)
+	}
+}
+
 func TestUIOpenRemoteSyncSetupDialogPrefillsCurrentVaultSetupFlow(t *testing.T) {
 	t.Parallel()
 
@@ -6280,6 +6315,95 @@ func TestUIRemoteSyncSetupCanPersistManualSyncMode(t *testing.T) {
 	}
 }
 
+func TestUIRemoveSelectedRemoteBindingActionClearsVaultBindingAndRecentRefs(t *testing.T) {
+	t.Parallel()
+
+	key := vault.MasterKey{Password: "correct horse battery staple"}
+	currentPath := filepath.Join(t.TempDir(), "current.kdbx")
+	writeKDBXMainTestFile(t, currentPath, vault.Model{
+		Entries: []vault.Entry{{
+			ID:       "remote-creds-1",
+			Title:    "WebDAV Sign-In",
+			Username: "tjulian",
+			Password: "token-1",
+			Path:     []string{"Crew", "Internet"},
+		}},
+		RemoteProfiles: []vault.RemoteProfile{{
+			ID:      "family-webdav",
+			Name:    "Family Vault",
+			Backend: vault.RemoteBackendWebDAV,
+			BaseURL: "https://dav.example.invalid/remote.php/dav",
+			Path:    "files/family/keepass.kdbx",
+		}},
+	}, key)
+
+	dir := t.TempDir()
+	u := newUIWithSession("desktop", &session.Manager{}, statePaths{
+		DefaultSaveAsPath: filepath.Join(dir, "vault.kdbx"),
+		RecentVaultsPath:  filepath.Join(dir, "recent-vaults.json"),
+		RecentRemotesPath: filepath.Join(dir, "recent-remotes.json"),
+		UIPreferencesPath: filepath.Join(dir, "ui-prefs.json"),
+	})
+	u.masterPassword.SetText(key.Password)
+	u.vaultPath.SetText(currentPath)
+	u.recentRemotes = []recentRemoteRecord{{
+		BaseURL:           "https://dav.example.invalid/remote.php/dav",
+		Path:              "files/family/keepass.kdbx",
+		LocalVaultPath:    currentPath,
+		RemoteProfileID:   "family-webdav",
+		CredentialEntryID: "remote-creds-1",
+		SyncMode:          string(appstate.SyncModeAutomaticOnOpenSave),
+	}}
+	if err := u.openVaultAction(); err != nil {
+		t.Fatalf("openVaultAction() error = %v", err)
+	}
+
+	if err := u.removeSelectedRemoteBindingAction(); err != nil {
+		t.Fatalf("removeSelectedRemoteBindingAction() error = %v", err)
+	}
+
+	if got := u.selectedVaultRemoteProfileID; got != "" {
+		t.Fatalf("selectedVaultRemoteProfileID = %q, want empty", got)
+	}
+	if got := u.selectedVaultRemoteCredentialEntryID; got != "" {
+		t.Fatalf("selectedVaultRemoteCredentialEntryID = %q, want empty", got)
+	}
+	if got := u.selectedVaultRemoteSyncMode; got != appstate.SyncModeManual {
+		t.Fatalf("selectedVaultRemoteSyncMode = %q, want manual", got)
+	}
+	if got := u.recentRemotes[0].RemoteProfileID; got != "" {
+		t.Fatalf("recentRemotes[0].RemoteProfileID = %q, want empty", got)
+	}
+	if got := u.recentRemotes[0].CredentialEntryID; got != "" {
+		t.Fatalf("recentRemotes[0].CredentialEntryID = %q, want empty", got)
+	}
+	if got := u.recentRemotes[0].SyncMode; got != "" {
+		t.Fatalf("recentRemotes[0].SyncMode = %q, want empty", got)
+	}
+	if got := u.state.StatusMessage; got != "Remote sync is no longer set up for this vault." {
+		t.Fatalf("StatusMessage = %q, want removal status", got)
+	}
+	if u.shouldShowDirectRemoteSyncShortcut() {
+		t.Fatal("shouldShowDirectRemoteSyncShortcut() = true, want false after removing binding")
+	}
+	if !u.shouldShowRemoteSyncSetupShortcut() {
+		t.Fatal("shouldShowRemoteSyncSetupShortcut() = false, want true after removing binding")
+	}
+
+	reopened := newUIWithSession("desktop", &session.Manager{})
+	reopened.masterPassword.SetText(key.Password)
+	reopened.vaultPath.SetText(currentPath)
+	if err := reopened.openVaultAction(); err != nil {
+		t.Fatalf("reopened.openVaultAction() error = %v", err)
+	}
+	if got := len(reopened.availableRemoteProfiles()); got != 0 {
+		t.Fatalf("len(reopened.availableRemoteProfiles()) = %d, want 0", got)
+	}
+	if got := len(reopened.availableRemoteCredentialEntries()); got != 0 {
+		t.Fatalf("len(reopened.availableRemoteCredentialEntries()) = %d, want 0", got)
+	}
+}
+
 func TestUISaveCurrentRemoteBindingActionPersistsBindingIntoVault(t *testing.T) {
 	t.Parallel()
 
diff --git a/vault/model.go b/vault/model.go
index 22e1cc1..31e171f 100644
--- a/vault/model.go
+++ b/vault/model.go
@@ -184,6 +184,17 @@ func (m *Model) UpsertEntry(entry Entry) {
 	m.Entries = append(m.Entries, cloneEntry(entry))
 }
 
+func (m *Model) RemoveEntryByID(id string) bool {
+	for i := range m.Entries {
+		if m.Entries[i].ID != id {
+			continue
+		}
+		m.Entries = append(m.Entries[:i], m.Entries[i+1:]...)
+		return true
+	}
+	return false
+}
+
 func (m *Model) EntryByID(id string) (Entry, error) {
 	for _, entry := range m.Entries {
 		if entry.ID == id {
@@ -204,6 +215,17 @@ func (m *Model) UpsertRemoteProfile(profile RemoteProfile) {
 	m.RemoteProfiles = append(m.RemoteProfiles, profile)
 }
 
+func (m *Model) RemoveRemoteProfileByID(id string) bool {
+	for i := range m.RemoteProfiles {
+		if m.RemoteProfiles[i].ID != id {
+			continue
+		}
+		m.RemoteProfiles = append(m.RemoteProfiles[:i], m.RemoteProfiles[i+1:]...)
+		return true
+	}
+	return false
+}
+
 func (m Model) RemoteProfileByID(id string) (RemoteProfile, error) {
 	for _, profile := range m.RemoteProfiles {
 		if profile.ID == id {